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We consider the Maximum 2-Club problem where one is given as input an undirected graph G = (V,E) and seeks a subset of vertices S of maximum size such that any pair of vertices in S is connected by a path of length at most 2 in the graph induced by S. This problem is a natural relaxation of the famous Maximum Clique problem where any pair of vertices must be connected by an edge. Maximum 2-Club has been well-studied and is known to be NP-complete even on split graphs. It can be solved exactly in O^*(1.62ⁿ) time, where n denotes the number of vertices of the input graph, while being polynomial-time solvable on several graph classes. Parameterized algorithms for structural parameters have also been considered, leading in particular to an algorithm with a double-exponential dependence in the parameter treewidth. Such an algorithm is actually the best one known for the larger parameter vertex cover size up to a constant in the exponent. We provide new results in both directions. We first prove that the double-exponential dependence for parameter vertex cover size is unavoidable under the Exponential Time Hypothesis (ETH). This answers a question left open by Hartung, Komusiewicz, Nichterlein and Suchỳ [Hartung et al., 2015]. Our result also implies that the problem cannot be solved in time sub-exponential in n even for split graphs. We then provide an exact algorithm for the problem restricted to chordal graphs, running in O^*(1.1996ⁿ) time, by reducing Maximum 2-Club on this class to Maximum Independent Set on arbitrary graphs with the same number of vertices. The same reduction shows that we can enumerate all maximum (and inclusion-wise maximal) 2-clubs of a chordal graph in O^*(3^{n/3}) = O^*(1.4423ⁿ) time. We conclude by providing a construction of split graphs with Ω(3^{n/3}/poly(n)) maximum2-clubs, for some polynomial poly showing that the bound for enumeration is essentially tight.